Angry, being pest-infested (5)
I believe the answer is:
ratty
'angry' is the definition.
(thesaurus)
'pest-infested' is the wordplay.
'pest' becomes 'rat' (rat can mean a nasty person).
'infested' becomes 'ty' (I am not sure about this - if you are sure you should give a lot more credence to this answer).
'rat'+'ty'='RATTY'
'being' acts as a link.
Can you help me to learn more?
(Other definitions for ratty that I've seen before include "Moley's friend" , "In a bad temper" , "water vole, literally" , "Irritable - Mole's friend!" , "One messing about in a boat" .)