Having knocked off Charlie, now make amends (5)
I believe the answer is:
atone
'make amends' is the definition.
(to atone is to make amends for a wrong deed)
I cannot understand how the rest of the clue works.
Can you help me to learn more?
(Other definitions for atone that I've seen before include "Recompense" , "Pay the price" , "Make redress" , "Turn away from sin and do penance" , "Make amends, being at one" .)