They look and sound agreeable (4)
I believe the answer is:
eyes
'they look' is the definition.
(I've seen this before)
I don't understand how the remainder of the clue works.
Can you help me to learn more?
(Other definitions for eyes that I've seen before include "Narrowly watches" , "Peacock's tail markings" , "Globular organs" , "Marks on potatoes" , "Closely looks at" .)