Two-thirds of Israel is upset about country's eastern border with this nation (5)
I believe the answer is:
syria
'nation' is the definition.
(Syria is an example)
I don't understand the remainder of the clue.
Can you help me to learn more?
(Other definitions for syria that I've seen before include "Arab republic, independent since 1946" , "Middle-East Republic" , "Near eastern country" , "Captain; omit; refuse container" , "Asian country" .)