Unnerves with babies' toys (7)
I believe the answer is:
rattles
I believe this clue is a double definition.
'unnerves' is the first definition.
(I've seen this in another clue)
'babies' toys' is the second definition.
(I've seen this in another clue)
'with' acts as a link.
(Other definitions for rattles that I've seen before include "Noisy toys for babies" , "Starlet (anag)" .)
I've seen this clue in The Daily Express.
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