Written in Sanskrit, he takes letter to Greeks (5)
I believe the answer is:
theta
'letter to greeks' is the definition.
(letter from the Greek alphabet)
'written in sanskrit he takes' is the wordplay.
'written in' indicates a hidden word.
'THETA' is hidden within 'sanskrit he takes'.
(Other definitions for theta that I've seen before include "letter from Athens" , "Letter to the Corinthians" , "Greek letter equivalent to th" , "classic character?" , "Letter before iota" .)