I calm us with arrangement that's harmonious (7)
I believe the answer is:
musical
'harmonious' is the definition.
(thesaurus)
'i calm us with arrangement' is the wordplay.
'i calm us' anagrams to 'MUSICAL'.
Though, I am not sure how the anagram is indicated.
'that's' is the link.
Can you help me to learn more?
(Other definitions for musical that I've seen before include "Annie maybe" , "Annie or Mame, say" , "Stage show; harmonious" , "Show with singing and dancing" , "Eg, Les Miserables" .)